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- W4385829238 abstract "Energy transfer between a sensitizer and a triplet annihilator-emitter system is a key process that dictates the design of a light energy upconversion system. Using a combination of steady-state and time-resolved emission experiments, we have now elucidated excited-state interactions between the rubrene dye and a perylene derivative (DBP), which are commonly employed in upconversion molecular assemblies. Quenching of rubrene emission with a concomitant increase in DBP emission in rubrene-DBP films confirms singlet-energy transfer with a singlet energy transfer efficiency as high as 94%. Under low-intensity (steady-state) excitation, the singlet excited state of rubrene acts as a primary donor in the Förster resonance energy transfer process. The rate constant of energy transfer as determined from emission lifetime measurements of rubrene-DBP films was 1.4 × 109 s–1. The factors that control the singlet energy transfer between excited rubrene and DBP and its role in designing light energy harvesting assemblies are discussed." @default.
- W4385829238 created "2023-08-16" @default.
- W4385829238 creator A5013108049 @default.
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- W4385829238 date "2023-08-15" @default.
- W4385829238 modified "2023-09-27" @default.
- W4385829238 title "Directing Singlet Excited Energy Flow in Rubrene-Perylene Dye (DBP) Films" @default.
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- W4385829238 doi "https://doi.org/10.1021/acs.jpcc.3c04003" @default.
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