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• W4385840127 endingPage "18759" @default.
• W4385840127 startingPage "18753" @default.
• W4385840127 abstract "The asymmetric difunctionalization of alkenes, a method transforming readily accessible alkenes into enantioenriched chiral structures of high value, has long been a focal point of organic synthesis. Despite tremendous efforts in this domain, it remains a considerable challenge to devise enantioselective oxidative dicarbofunctionalization of alkenes, even though these transformations can utilize stable and unfunctionalized functional group donors. In this context, we report herein a photoelectrocatalytic method for the enantioselective heteroarylcyanation of aryl alkenes, which employs unfunctionalized heteroarenes through C–H functionalization. The photoelectrochemical asymmetric catalysis (PEAC) method combines photoredox catalysis and asymmetric electrocatalysis to facilitate the formation of two C–C bonds operating via hydrogen (H2) evolution and obviating the need for external chemical oxidants." @default.
• W4385840127 created "2023-08-16" @default.
• W4385840127 creator A5051163798 @default.
• W4385840127 creator A5067738552 @default.
• W4385840127 date "2023-08-15" @default.
• W4385840127 modified "2023-10-17" @default.
• W4385840127 title "Photoelectrochemical Asymmetric Catalysis Enables Enantioselective Heteroarylcyanation of Alkenes via C–H Functionalization" @default.
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• W4385840127 doi "https://doi.org/10.1021/jacs.3c07146" @default.
• W4385840127 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37581933" @default.
• W4385840127 hasPublicationYear "2023" @default.
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