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- W4385840904 abstract "Electrocatalytic nitrate reduction (ENR) to N2 is a promising approach to eliminate nitrate (NO3--N) for solving the eutrophication of water bodies, but it still faces the significant challenge of exploiting efficient electrocatalysts. Herein, a three-dimensional self-supporting Cu-CoOx/CC hybrid was fabricated based on the oxygen vacancy-rich and interfacial engineering strategies for the purpose of the effective electrochemical conversion of NO3--N to N2. The fabricated hybrid catalyst possessed a unique structure of nanoporous, oxygen vacancy-rich and multi-interface. More importantly, it was effectively competent for the selective reduction of NO3--N to N2. Under the optimized conditions (initial NO3--N concentration: 50 mg L-1; pH: 7.0; current density: 20 mA cm-2), the Cu-CoOx/CC exhibited 92.3% NO3--N removal efficiency and 57.8 % N2 selectivity after 3 h electrolysis treatment. Moreover, due to the synergistic coupling of Cu and CoOx, the electrocatalytic NO3--N reduction performances and expected intermediates can be regulated. This work could provide a valuable guidance for the synthesis of highly active and selective ERN hybrid electrocatalysts and the pollution control of water eutrophication." @default.
- W4385840904 created "2023-08-16" @default.
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- W4385840904 date "2023-12-01" @default.
- W4385840904 modified "2023-10-17" @default.
- W4385840904 title "Oxygen vacancy-rich nanoporous Cu-CoO /CC hybrid catalyst for controllable electrocatalytic reduction of nitrate" @default.
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- W4385840904 doi "https://doi.org/10.1016/j.seppur.2023.124815" @default.
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