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• W4385841109 abstract "Introducing carbon vacancies (Vc) is an efficient strategy that can improve the catalytic activity of carbon materials. However, the understanding in the efficacy and mechanism of Vc in peroxymonosulfate (PMS) adsorption and activation to degrade pollutants was inexplicit. Herein, Vc was introduced into the catalyst (PB-Mn-X) via etching and heat treatment for Prussian blue, and four PB-Mn-Xs with different Vc contents were used to investigate the performance and mechanism. As a result, PB-Mn-X had excellent catalytic performance and good cycling stability, removing 93.7% Acetaminophen (APAP) within 10 min and being almost independent of pH value. Quenching results and electron paramagnetic resonance (EPR) technology confirmed that PB-Mn-X/PMS system was a surface oxidation mechanism with four reactive oxygen species (SO4•–, •OH, O2•–, and 1O2). The presence of Vc enhanced the PMS adsorption, thus building an electron-deficient surface on material. APAP with electron-rich groups was easy adsorbed on such a surface, which boosted the efficiently and rapidly APAP degradation. In addition, the actual application performance of PB-Mn-X/PMS system was also assessed. This work provides favorable insights to advance the research on the catalytic efficiency and mechanism of Vc on activated PMS." @default.
• W4385841109 created "2023-08-16" @default.
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• W4385841109 date "2023-12-01" @default.
• W4385841109 modified "2023-10-17" @default.
• W4385841109 title "Applying the carbon vacancy-enhanced catalyst as the surface reactor for peroxymonosulfate activation and efficient Acetaminophen degradation: Performance and mechanism" @default.
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• W4385841109 doi "https://doi.org/10.1016/j.seppur.2023.124811" @default.
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