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- W4385872877 abstract "Abstract In order to diminish environmental issues such as global warming due to increased carbo dioxide (CO 2 ) emissions, considerable efforts have been made in the research community. Photocatalytic hydrogen (H 2 ) production is a very important way towards this goal, since sunlight is an abundant source of energy and H 2 is a clean fuel, producing no greenhouse gases. Inexpensive, stable and non‐toxic carbon dots were easily synthesized and used as photosensitizers in water in the presence of a series of molecular cobalt catalysts ( CoTSC ). The catalysts were thiosemicarbazone‐based complexes able to transfer electrons for hydrogen evolution reaction. Under visible light irradiation, the nitrogen‐doped carbon dots ( NCdots ) transfer the photoexcited electrons to the catalyst, producing an activity of 358 μmol g NCdot −1 h −1 (TON Co =570) for CoTSC−N(CH 3 ) 2 CN after 24 h of irradiation. These types of molecular catalysts display great activity and stability in combination with the easily synthesized and modified carbon dot materials." @default.
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- W4385872877 date "2023-09-13" @default.
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- W4385872877 title "A series of cobalt bis(thiosemicarbazone) catalysts for effective photocatalytic hydrogen evolution reaction" @default.
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- W4385872877 doi "https://doi.org/10.1002/ejic.202300352" @default.
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