Matches in SemOpenAlex for { <https://semopenalex.org/work/W4385879475> ?p ?o ?g. }
- W4385879475 endingPage "101734" @default.
- W4385879475 startingPage "101734" @default.
- W4385879475 abstract "Solar-to-chemical energy conversion through artificial photosynthesis is an ideal route to address the global energy crisis and realize carbon neutrality in the future. Over the past decade, two-dimensional conjugated polymer frameworks (2D CPFs), including conjugated microporous polymers, covalent organic frameworks, and covalent triazine frameworks, have emerged as a promising class of photocatalysts for solar fuel generation. They exhibit highly tunable chemical and optoelectronic structures which can be precisely controlled at the molecular level. Meanwhile, the 2D planar structure with in-plane periodicity offers many unique features for solar-driven catalytic energy conversion, including large surface areas, high absorption coefficients, efficient charge transport, and facile formation of heterostructures. In addition, their surface active sites can be rationally constructed from numerous molecular building blocks to optimize their photocatalytic performances. Herein, we comprehensively summarize recent progress in developing 2D CPFs for solar fuel generation from water, including photocatalytic overall water splitting, hydrogen peroxide production, carbon dioxide reduction, and nitrogen fixation. Basic principles in these photocatalytic reactions are described. In-depth insights into the structure-property relationships between 2D CPFs and their reaction mechanisms are discussed in detail. Moreover, recent advances in applications of 2D CPFs in photoelectrochemical energy conversion are also highlighted. Finally, the remaining challenges and research opportunities for the future development of efficient 2D CPFs toward solar fuel generation are presented." @default.
- W4385879475 created "2023-08-17" @default.
- W4385879475 creator A5067487673 @default.
- W4385879475 creator A5073216396 @default.
- W4385879475 date "2023-10-01" @default.
- W4385879475 modified "2023-10-13" @default.
- W4385879475 title "Two‐dimensional conjugated polymer frameworks for solar fuel generation from water" @default.
- W4385879475 cites W1238502700 @default.
- W4385879475 cites W1799122600 @default.
- W4385879475 cites W1930734459 @default.
- W4385879475 cites W1947688540 @default.
- W4385879475 cites W1965344362 @default.
- W4385879475 cites W1969929163 @default.
- W4385879475 cites W1971113415 @default.
- W4385879475 cites W1971865766 @default.
- W4385879475 cites W1974659797 @default.
- W4385879475 cites W1977892176 @default.
- W4385879475 cites W1989703096 @default.
- W4385879475 cites W2010571276 @default.
- W4385879475 cites W2025806519 @default.
- W4385879475 cites W2033067297 @default.
- W4385879475 cites W2034290864 @default.
- W4385879475 cites W2034926370 @default.
- W4385879475 cites W2040115060 @default.
- W4385879475 cites W2042492216 @default.
- W4385879475 cites W2043885009 @default.
- W4385879475 cites W2050612192 @default.
- W4385879475 cites W2052600292 @default.
- W4385879475 cites W2057594988 @default.
- W4385879475 cites W2068655749 @default.
- W4385879475 cites W2079666951 @default.
- W4385879475 cites W2105991801 @default.
- W4385879475 cites W2116809081 @default.
- W4385879475 cites W2123708609 @default.
- W4385879475 cites W2131415600 @default.
- W4385879475 cites W2133213134 @default.
- W4385879475 cites W2134491231 @default.
- W4385879475 cites W2143194153 @default.
- W4385879475 cites W2143415304 @default.
- W4385879475 cites W2150399639 @default.
- W4385879475 cites W2252538303 @default.
- W4385879475 cites W2269220428 @default.
- W4385879475 cites W2283290883 @default.
- W4385879475 cites W2295326161 @default.
- W4385879475 cites W2312573052 @default.
- W4385879475 cites W2317411269 @default.
- W4385879475 cites W2328465686 @default.
- W4385879475 cites W2340212768 @default.
- W4385879475 cites W2412520413 @default.
- W4385879475 cites W2473791518 @default.
- W4385879475 cites W2571928238 @default.
- W4385879475 cites W2572667976 @default.
- W4385879475 cites W2592046628 @default.
- W4385879475 cites W2593425684 @default.
- W4385879475 cites W2597651742 @default.
- W4385879475 cites W2612385653 @default.
- W4385879475 cites W2620180261 @default.
- W4385879475 cites W2622516231 @default.
- W4385879475 cites W2722013064 @default.
- W4385879475 cites W2736305270 @default.
- W4385879475 cites W2737308721 @default.
- W4385879475 cites W2741257603 @default.
- W4385879475 cites W2748311356 @default.
- W4385879475 cites W2753723386 @default.
- W4385879475 cites W2755269103 @default.
- W4385879475 cites W2757404001 @default.
- W4385879475 cites W2763525349 @default.
- W4385879475 cites W2768372190 @default.
- W4385879475 cites W2772283135 @default.
- W4385879475 cites W2781636403 @default.
- W4385879475 cites W2784735527 @default.
- W4385879475 cites W2787956937 @default.
- W4385879475 cites W2791723510 @default.
- W4385879475 cites W2793388266 @default.
- W4385879475 cites W2796379964 @default.
- W4385879475 cites W2801184875 @default.
- W4385879475 cites W2801639961 @default.
- W4385879475 cites W2803544914 @default.
- W4385879475 cites W2806955329 @default.
- W4385879475 cites W2809379320 @default.
- W4385879475 cites W2877882896 @default.
- W4385879475 cites W2884894404 @default.
- W4385879475 cites W2889369905 @default.
- W4385879475 cites W2893029634 @default.
- W4385879475 cites W2893418494 @default.
- W4385879475 cites W2893495355 @default.
- W4385879475 cites W2896375080 @default.
- W4385879475 cites W2896858547 @default.
- W4385879475 cites W2897927724 @default.
- W4385879475 cites W2900060043 @default.
- W4385879475 cites W2900456365 @default.
- W4385879475 cites W2901001562 @default.
- W4385879475 cites W2902266031 @default.
- W4385879475 cites W2903719108 @default.
- W4385879475 cites W2908301765 @default.
- W4385879475 cites W2913379862 @default.
- W4385879475 cites W2914840694 @default.
- W4385879475 cites W2918073057 @default.