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- W4385955559 abstract "Abstract The strong correlations between electrons in Mott insulator materials may produce highly entangled many-body states with unconventional emergent excitations. The signatures of such excitations, if any, are commonly believed to be observable only at low temperatures. Here, we challenge this common belief and show using terahertz time-domain spectroscopy that exotic carriers exist even at room temperature in TbInO 3 , a candidate material for realizing a low-temperature quantum spin-liquid phase. In particular, over the entire temperature range of 1.5–300 K, we observe a quadratic frequency dependence in the real part of the in-plane optical conductivity as well as Fano asymmetry of an optical phonon mode strongly interacting with the excitation continuum. These features are robust even under external magnetic fields of up to 7 T. Our data confirm the presence of emergent charge carriers within the Mott charge gap of TbInO 3 , suggesting that it is possible to probe and manipulate highly entangled quantum many-body states at room temperature." @default.
- W4385955559 created "2023-08-18" @default.
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- W4385955559 date "2023-08-17" @default.
- W4385955559 modified "2023-10-17" @default.
- W4385955559 title "Unconventional room-temperature carriers in the triangular-lattice Mott insulator TbInO3" @default.
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- W4385955559 doi "https://doi.org/10.1038/s41567-023-02174-5" @default.
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