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• W4385982010 abstract "This work reports the first comprehensive observation for the distribution of 233U and 236U in sediment cores collected from the major basins across the Baltic Sea. In addition to 233U and 236U, this study encompassed the analysis of 137Cs, 239Pu and 240Pu in the same sediment core samples. Depth profiles of 233U and 236U in Baltic Sea sediments indicate that 233U or global fallout (GF)-derived 236U is a useful time marker, in addition to 239+240Pu, to identify the onset of the Anthropocene epoch. Based on the cumulative areal inventories reported previously for water columns and investigated herein for sediment cores, our estimated overall inventories of 233U and 236U in the present Baltic Sea water and sediment are about 18 ± 6 g and 2010 ± 547 g, respectively, with >80 % accumulated in the Baltic seabed (i.e., 16 ± 6 g of 233U and 1694 ± 522 g of 236U, respectively). The total budget for nuclear reactor (NR)-derived 236U in the Baltic seabed is estimated to be 683 ± 223 g. Despite covering only 13 % of the total area, the hypoxic regions (325 ± 64 g) reserve a nearly equivalent amount of NR-derived 236U as the oxygenated regions (358 ± 159 g), highlighting the significance of the hypoxic regions in retaining NR-derived 236U. With a multi-radionuclide approach, this work contributes to a more thorough understanding on distribution and accumulation of anthropogenic uranium in the Baltic Sea." @default.
• W4385982010 created "2023-08-19" @default.
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• W4385982010 date "2023-11-01" @default.
• W4385982010 modified "2023-10-12" @default.
• W4385982010 title "Stratigraphic records and inventories of anthropogenic 233U and 236U in Baltic Sea sediments" @default.
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• W4385982010 doi "https://doi.org/10.1016/j.scitotenv.2023.166402" @default.
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