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- W4386003458 abstract "Development of photocatalytic membrane with antifouling, permeability, selectivity and reusability is highly desired for water treatment. Herein, an imprinted poly-3,4-ethylenedioxythiophene/oxygen-rich bismuth chloride oxide heterojunction embedded membrane (I-PEDOT/Bi12O17Cl2−M) with good self-cleaning and recyclability was fabricated by integrating surface corrosion and imprinting strategy. The introduction of imprinting technology endowed Z-type heterojunction (composed of Bi12O17Cl2 nanosheets and PEDOT) with imprinted cavities which possessed good selective adsorption ability for target pollutant (tetracycline, TC). Compared with pure nanosheets (Bi12O17Cl2) and non-imprinted nanosheets photocatalyst (NI-PEDOT/Bi12O17Cl2), the selectivity coefficient of I-PEDOT/Bi12O17Cl2−M were 3.35 and 2.01, respectively. Importantly, the corrosive solvent (NMP) changed the surface pore structure of polyvinylidene fluoride (PVDF), which firmly stuck the two-dimensional I-PEDOT/Bi12O17Cl2 in the surface pore of PVDF base membrane, avoiding the catalyst encapsulation issue of conventional methods and fully exposing the active sites. Therefore, I-PEDOT/Bi12O17Cl2−M exhibited good catalytic activity and stability. Particularly, the pure water flux and TC flux reached 4620 L/m2·h and 3580 L/m2·h, respectively. This study provides a new strategy for reasonable design of photocatalytic membrane with high permeability and good selectivity." @default.
- W4386003458 created "2023-08-20" @default.
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- W4386003458 date "2023-10-01" @default.
- W4386003458 modified "2023-10-07" @default.
- W4386003458 title "Integrating surface corrosion and imprinting strategy into PEDOT/Bi12O17Cl2 heterojunction embedded membrane aims to high permeability and selectivity" @default.
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- W4386003458 doi "https://doi.org/10.1016/j.surfin.2023.103303" @default.
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