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- W4386023102 abstract "Low dimensional perovskite-inspired materials with self-tapped exciton (STE) emission have stimulated a surge of cutting-edge research in optoelectronics. Despite numerous efforts on developing versatile low-dimensional perovskite-inspired materials with efficient STE emissions, there is little emphasis on the intrinsic dynamics of STE-based broad emission in these materials. Here, we investigated the excited state dynamics in zero-dimensional (0D) Cs2ZrCl6 nanocrystals (NCs) with efficient blue STE emission. By using femtosecond transient absorption (fs-TA) spectroscopy, the ultrafast STE formation process within 400 fs is directly observed. Then, the formed STEs relax to an intermediate STE state with a lifetime of ∼180 ps before reaching the emissive STE state with a lifetime of ∼15 μs. Our work offers a comprehensive and precise dynamic picture of STE emission in low-dimensional metal halides and sheds light on extending their potential applications." @default.
- W4386023102 created "2023-08-22" @default.
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- W4386023102 date "2023-08-21" @default.
- W4386023102 modified "2023-10-18" @default.
- W4386023102 title "Nature of Self-Trapped Exciton Emission in Zero-Dimensional Cs<sub>2</sub>ZrCl<sub>6</sub> Perovskite Nanocrystals" @default.
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- W4386023102 doi "https://doi.org/10.1021/acs.jpclett.3c01878" @default.
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