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• W4386051840 abstract "The design and synthesis of air-stable single-molecule magnets (SMMs) with large effective barriers of magnetic reversal and remarkably slow relaxation times are challenging. The design and synthesis of air-stable complexes with large effective magnetic reversal barriers and remarkably slow relaxation times are challenging in the field of SMMs. Herein, we present an air-stable hexagonal bipyramid [DyIII(bpyN4)(Ph3SiO)2](BPh4) (1) (bpyN4 = neutral hexaaza macrocyclic Schiff base ligand derived of 6,6′-diformyl-2,2′-bipyridyl and triethylenetetramine). The magnetic data demonstrate that the complex shows zero-field SMM behavior with magnetic hysteresis loops up to 13 K and an effective barrier of 584 K for 1. The experimental effective barrier is close to the energy of the first excited Kramers doublet (EKD1) obtained from ab initio calculations." @default.
• W4386051840 created "2023-08-23" @default.
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• W4386051840 date "2023-08-21" @default.
• W4386051840 modified "2023-10-17" @default.
• W4386051840 title "Macrocyclic Hexagonal Bipyramidal Dy(III)-Based Single-Molecule Magnets with a <i>D</i>_6<i>h</i> Symmetry" @default.
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• W4386051840 doi "https://doi.org/10.1021/acs.cgd.3c00813" @default.
• W4386051840 hasPublicationYear "2023" @default.
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