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- W4386052728 abstract "Birnessite plays a crucial role in regulating the fate of contaminants in soil, which is affected by the crystal structure of birnessite. In this study, the transformation of triclinic birnessite to hexagonal birnessite was examined at various pH values, and their reactivity towards norfloxacin was investigated. The findings indicate that the conversion from triclinic birnessite to hexagonal birnessite occurs under pH conditions lower than 7. The lower of the solution pH where the birnessite formed, the higher the surface reactivity. Throughout the transformation process, the migration of Mn3+ and the increased interlayer protons generated more reactive oxygen species, which enhanced the surface reactivity towards norfloxacin. Specifically, at a conversion pH of 1, the norfloxacin removal rate significantly increases from 14% to 97% compared to triclinic birnessite. The mechanism of norfloxacin removal by triclinic and hexagonal birnessite is illustrated. These findings provide valuable insights into the dynamic transformation of birnessites in aqueous environments with varying pH values and their impact on norfloxacin removal." @default.
- W4386052728 created "2023-08-23" @default.
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- W4386052728 date "2023-11-01" @default.
- W4386052728 modified "2023-10-16" @default.
- W4386052728 title "The pH-sensitive transformation of birnessite and its effect on the fate of norfloxacin" @default.
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- W4386052728 doi "https://doi.org/10.1016/j.chemosphere.2023.139932" @default.
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