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• W4386067774 abstract "Two-dimensional multiferroic materials are highly sought after due to their huge potential for applications in nanoelectronic and spintronic devices. Here, we predict, based on first-principle calculations, a single-phase triferroic where three ferroic orders---ferromagnetism, ferroelectricity, and ferroelasticity---coexist simultaneously in the hole doped ${mathrm{GdCl}}_{2}$ monolayer (a ferromagnetic semiconductor). This is achieved by substituting 1/3rd of the ${mathrm{Gd}}^{2+}$ ions with ${mathrm{Eu}}^{2+}$ in the hexagonal structure of the ${mathrm{GdCl}}_{2}$ monolayer. The resulting metallic state undergoes a bond-centered charge ordering driving a distortion in the hexagonal structure, making it semiconducting again and ferroelastic. Further, the lattice distortion accompanied by a breaking of the lattice centrosymmetry renders a noncentrosymmetric charge distribution, which makes the monolayer ferroelectric, at the same time. The two ferroic orders, ferroelectricity and ferroelasticity, present in the Eu-substituted ${mathrm{GdCl}}_{2}$ monolayer are found to be strongly coupled, making it a promising candidate for device applications. The Eu-substituted monolayer remains a ferromagnetic semiconductor with a large $4f$ magnetic moment just like the parent monolayer and possesses an even higher (out-of-plane) magnetic anisotropy energy than its pristine counterpart as desired for two-dimensional magnets to have high transition temperature." @default.
• W4386067774 created "2023-08-23" @default.
• W4386067774 creator A5012339956 @default.
• W4386067774 creator A5023085497 @default.
• W4386067774 date "2023-08-22" @default.
• W4386067774 modified "2023-09-25" @default.
• W4386067774 title "Two-dimensional rare-earth halide based single-phase triferroic" @default.
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• W4386067774 doi "https://doi.org/10.1103/physrevb.108.l081116" @default.
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