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- W4386087452 endingPage "145612" @default.
- W4386087452 startingPage "145612" @default.
- W4386087452 abstract "Hydrogen (H2) is regarded as a novel energy carrier with huge development potential, and it will be essential in future clean energy systems. Given the existing challenges in direct H2 storage and delivery, effective H2 storage carriers, such as formic acid, for on-site H2 production have received widespread attention. Recently, supported heterogeneous catalysts have made significant progress in formic acid decomposition (FAD) toward H2, to overcome the shortcomings of homogeneous catalysts’ poor stability, separation difficulty, and serious pollution. Herein, we summarize the catalytic mechanism of H2 production from FAD catalyzed by heterogeneous catalysts, thoroughly discuss the optimization of FAD performance based on MSI regulation according to metal (size, composition, and atomic arrangement), support (composition, surface modification, heteroatom doping, and confinement), and treatment (heat and plasma), as well as propose a rational design and precise construction approach for efficient FAD catalytic structures according to MSI. This review improves the development of the ideal heterogeneous FAD catalysts, to meet the demand for on-site H2 production in the future green energy system." @default.
- W4386087452 created "2023-08-24" @default.
- W4386087452 creator A5012219750 @default.
- W4386087452 creator A5013206214 @default.
- W4386087452 creator A5034266315 @default.
- W4386087452 creator A5043839950 @default.
- W4386087452 creator A5066221855 @default.
- W4386087452 creator A5076759275 @default.
- W4386087452 date "2023-10-01" @default.
- W4386087452 modified "2023-09-26" @default.
- W4386087452 title "Metal-support interactions in heterogeneous catalytic hydrogen production of formic acid" @default.
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