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- W4386099571 abstract "The approach for promoting the tunable photochemical properties of NiMOF for catalytic applications has been recognized as a smart choice for solar water splitting. However, the major concern is the low specific surface area (SSA). The present approach has specifically resolved this problem by tuning the nature of the surface of NiMOF by anchoring with ultranano-sized CeO2. The CeO2 (111) plane has a strong electron migrating affinity, and hence, the heterojunction significantly facilitates and directs the photoinduced electrons toward the reaction centers. In addition, the existence of NiMOF with switchable valence states as catalytic centers in the heterojunction also efficiently catalyzes the proton reduction. The enhancement in SSA of NiMOF and the surface tuning with ultranano-sized CeO2 are the key reasons for the observed higher activity (2.14 mmol/g/h) of the 0.2:1-CeO2@NiMOF hybrid composite with a high AQE value (18.82% at 320 nm). The results obtained are compared and found to be highly competitive with respect to high standard recent reports." @default.
- W4386099571 created "2023-08-24" @default.
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- W4386099571 date "2023-08-23" @default.
- W4386099571 modified "2023-10-15" @default.
- W4386099571 title "Tuning and Sustainment of High Surface Area of Nano CeO<sub>2</sub>-Anchored NiMOF Flake Heterojunctions for Efficient Photocatalytic Hydrogen Generation" @default.
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- W4386099571 doi "https://doi.org/10.1021/acs.energyfuels.3c02009" @default.
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