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- W4386156750 abstract "Abstract Supported Pd catalyst is an important noble metal material in recent years due to its high catalytic performance in CO 2 hydrogenation. An fluidized-bed plasma assisted atomic layer deposition (FP-ALD) process is reported to fabricate Pd nanoparticle catalyst over γ-Al 2 O 3 or Fe 2 O 3 /γ-Al 2 O 3 support, using palladium hexafluoroacetylacetonate as the Pd precursor and H 2 plasma as counter-reactant. Scanning transmission electron microscopy exhibits that high-density Pd nanoparticles are uniformly dispersed over Fe 2 O 3 /γ-Al 2 O 3 support with an average diameter of 4.4 nm. The deposited Pd-Fe 2 O 3 /γ-Al 2 O 3 shows excellent catalytic performance for CO 2 hydrogenation in a dielectric barrier discharge reactor. Under a typical condition of H 2 to CO 2 ratio of 4 in the feed gas, the discharge power of 19.4 W, and gas hourly space velocity of 10000 h − 1 , the conversion of CO 2 is as high as 16.3% with CH 3 OH and CH 4 selectivities of 26.5% and 3.9%, respectively." @default.
- W4386156750 created "2023-08-26" @default.
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- W4386156750 date "2023-08-25" @default.
- W4386156750 modified "2023-10-16" @default.
- W4386156750 title "Preparation of palladium-based catalyst by plasma-assisted atomic layer deposition and its applications in CO2 hydrogenation reduction" @default.
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- W4386156750 doi "https://doi.org/10.21203/rs.3.rs-3274623/v1" @default.
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