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- W4386157008 abstract "Dual nickel photoredox catalysis conditions have been developed for the decarboxylative cross-coupling of aryl halides and carboxylic acids containing fully substituted α-carbons, a valuable but challenging substrate class for C(sp2)–C(sp3) bond-forming reactions. High-throughput experimentation identified Ni(TMHD)2 as the optimal precatalyst for this reaction in contrast to the nickel-bipyridyl complexes typically employed in decarboxylative couplings, which predominantly furnished undesired C–O products. Computational work provides insight into the potential mechanistic underpinnings for the C–C vs C–O selectivity for the nickel-diketonate complex." @default.
- W4386157008 created "2023-08-26" @default.
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- W4386157008 date "2023-08-25" @default.
- W4386157008 modified "2023-10-14" @default.
- W4386157008 title "Unlocking Tertiary Acids for Metallaphotoredox C(sp<sup>2</sup>)–C(sp<sup>3</sup>) Decarboxylative Cross-Couplings" @default.
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- W4386157008 doi "https://doi.org/10.1021/acscatal.3c03353" @default.
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