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- W4386191151 abstract "Abstract The development of low cost‐effective and highly efficient heterogeneous electrocatalysts is most appreciable in the research community. A newly designed microporous organic‐inorganic hybrid iron cobalt phosphonate (FeCoDPAM) is synthesized using diphenylphosphinamide as an organophosphorus ligand through a hydrothermal pathway without any template. To synthesize N, P‐codoped bimetallic oxides (NP/FeCoO350, NP/FeCoO550, and NP/FeCoO750), the as‐synthesized material FeCoDPAM has undergone pyrolysis at three different temperatures, i. e ., 350, 550, 750 °C, respectively. The high specific surface area and a regular microporous array of N, P‐codoped iron cobalt oxide (NP/FeCoO350) material provide excellent oxygen evolution reaction (OER) activity. The NP/FeCoO350 material catalyzes OER with the overpotential of 331 mV at a current density of 10 mAcm −2 and Tafel slope of 56.7 mV dec −1 in 1.0 M KOH solution. The inclusion of iron in the cobalt phosphonate framework can change the electronic structure, and electron transfer can be feasible to the d ‐orbital of cobalt. Due to the doping of heteroatoms such as N and P into the bimetallic oxide matrix, a synergistic effect can occur, which is the driving force for the efficient electrocatalytic OER activity. Also, the FeCoO350 displays stability with outstanding oxidative current up to 50 h time in chronoamperometry measurement." @default.
- W4386191151 created "2023-08-27" @default.
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- W4386191151 date "2023-09-28" @default.
- W4386191151 modified "2023-10-09" @default.
- W4386191151 title "Iron cobalt phosphonate derived heteroatom doped metal oxides as superior electrocatalysts for water oxidation reaction" @default.
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- W4386191151 doi "https://doi.org/10.1002/cctc.202300731" @default.
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