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• W4386208117 abstract "With the advent of globalization, the upsurge of lithium-ion battery (LIB) production and generation of spent batteries impose a severe threat as hazardous e-waste and resource sustainability of crucial elements like cobalt and lithium. Herein, we propose one-step regeneration of cobalt oxide (RCO) from cycled LiCoO 2 (LCO)-type cathode via carbon anode-assisted reduction. The inherent structural changes resulting in high irreversibility are minimized in conversion-type mixed-phase recycled cobalt oxide anode due to less Li-ion consumption and stable SEI formation during initial cycles. Replacement of conventional Cu-foil current collector with carbon-fiber (CF) based freestanding electrode further enhances the Li-ion storage capacity with overall active material utilization, accommodating volume changes in the internal void spaces and providing mechanical stability. Electrochemistry reveals that RCO@CF and RCO@Cu deliver an initial discharge capacity of 3800 mAh g −1 and 1432 mAh g −1 at 30 mAg −1 with 77% and 64% coulombic efficiency that becomes ∼97% in the following cycles. Besides, RCO@CF shows an average discharge capacity of 730 mAh g −1 at 300 mA g −1 over 300 cycles, which is ∼2.7 times that of recycled graphite anode (270 mAh g −1 ). The sustainable recycling strategy described herein rejuvenates the cycled LCO-type cathode as an appealing anode material for LIBs." @default.
• W4386208117 created "2023-08-28" @default.
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• W4386208117 date "2023-09-01" @default.
• W4386208117 modified "2023-09-30" @default.
• W4386208117 title "Unravelling Li-ion Storage Capability of Cobalt Oxide Anode Recovered from Spent LiCoO₂ Cathode via Carbothermal Reduction" @default.
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• W4386208117 doi "https://doi.org/10.1149/1945-7111/acf480" @default.
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