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- W4386226673 abstract "Electrochemical upcycling of plastic waste to high-value chemicals is an ideal approach for the valorization of waste resources. In this study, we report the electro-reforming of polyethylene terephthalate (PET) plastic hydrolysate to valuable formate and hydrogen. Pd-deposited hierarchical aligned NiTe nanoarrays on Ni foam (Pd-NiTe/NF) is developed for oxidation of PET hydrolysate at anode and hydrogen evolution at cathode, with the overpotentials of 0.019 and 1.35 V at 10 and 100 mA cm-2, respectively. In co-electrolysis system, the Pd-NiTe/NF exhibits high Faradaic efficiencies for concurrent production of value-added formate (95.6%) and H2 (98.6%). The high activity and stability of Pd-NiTe/NF can be ascribed to that the interfacial heterostructures by incorporating Pd atoms and the strongly interfacial electronic interactions of between Pd and NiTe can synergistically promote PET-derived ethylene glycol to formate oxidation and hydrogen evolution. This work shows promising prospect in electro-reforming PET plastic waste to valuable chemicals." @default.
- W4386226673 created "2023-08-29" @default.
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- W4386226673 date "2024-01-01" @default.
- W4386226673 modified "2023-10-17" @default.
- W4386226673 title "Electrocatalytic Upcycling of Polyethylene Terephthalate Plastic to Formic Acid Coupled with Energy-Saving Hydrogen Production over Hierarchical Pd-Doped NiTe Nanoarrays" @default.
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- W4386226673 doi "https://doi.org/10.1016/j.apcatb.2023.123236" @default.
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