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• W4386282810 abstract "Past decade has witnessed the great improvement of carbon-based dual-single metal-site electrocatalysts. However, there are rare reports exploring the enhanced effect of a nonmetallic “dual-site” in carbon-based catalysts. Herein, a “H3BO3 template” method is proposed to fabricate highly active B–S pairs dispersed on a hierarchically microporous/mesoporous carbon matrix to electrochemically synthesize hydrogen peroxide by two-electron oxygen reduction reaction. Under the synergistic effect of B–S pairs and advantageous nanostructures, the catalytic performance outperforms the reported metal-free carbon catalysts in alkaline electrolytes, especially, with a high HO2– selectivity of 90–94% at a wide potential range of 0.3–0.7 V versus reversible hydrogen electrode (RHE) using a rotating ring-disk electrode, Faradaic efficiency of over 90% during 11 h stability testing, and high mass activity of 756 mmol gcatalyst–1 h–1 in a flow cell. Density functional theory demonstrates that the carbon atoms nearby B–S pairs exhibit predominant catalytic sites. This paper proposes a new approach to distinctly improve the catalytic performance by dual heteroatom pairs." @default.
• W4386282810 created "2023-08-31" @default.
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• W4386282810 date "2023-08-30" @default.
• W4386282810 modified "2023-10-17" @default.
• W4386282810 title "Boron–Sulfur Pairs for Highly Active 2e^– Oxygen Reduction Reaction to Electrochemically Synthesize Hydrogen Peroxide" @default.
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• W4386282810 doi "https://doi.org/10.1021/acssuschemeng.3c02620" @default.
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