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• W4386332531 abstract "Abstract Solar‐driven biohybrid systems that produce chemical energy are a valuable objective in ongoing research. However, reactive oxygen species (ROS) that accompany nanoparticle production under light radiation severely affect the efficiency of biohybrid systems. In this study, we successfully constructed a two‐hybrid system, Shewanella oneidensis ‐CdS and S. oneidensis ‐CdS@Fe 3 O 4 , in a simple, economical, and gentle manner. With the Fe 3 O 4 coating, ROS were considerably eliminated; the hydroxyl radical, superoxide radical, and hydrogen peroxide contents were reduced by 66.7%, 65.4%, and 72%, respectively, during light‐driven S. oneidensis ‐CdS hydrogen production. S. oneidensis ‐CdS@Fe 3 O 4 showed a 2.6‐fold higher hydrogen production (70 h) than S. oneidensis ‐CdS. Moreover, the S. oneidensis ‐CdS system produced an additional 367.8 μmol g‐dcw −1 (70 h) of hydrogen compared with S. oneidensis during irradiation. The apparent quantum efficiencies of S. oneidensis ‐CdS and S. oneidensis ‐CdS@Fe 3 O 4 were 6.2% and 11.5%, respectively, exceeding values previously reported. In conclusion, a stable nanozyme coating effectively inhibited the cytotoxicity of CdS nanoparticles, providing an excellent production environment for bacteria. This study provides a rational strategy for protecting biohybrid systems from ROS toxicity and contributes to more efficient solar energy conversion in the future." @default.
• W4386332531 created "2023-09-01" @default.
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• W4386332531 date "2023-09-22" @default.
• W4386332531 modified "2023-10-17" @default.
• W4386332531 title "Fe₃O₄ nanozyme coating enhances light‐driven biohydrogen production in self‐photosensitized <i>Shewanella oneidensis</i>‐CdS hybrid systems" @default.
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• W4386332531 doi "https://doi.org/10.1002/biot.202300084" @default.
• W4386332531 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37651217" @default.
• W4386332531 hasPublicationYear "2023" @default.
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