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• W4386346563 abstract "Single-molecule magnets are molecular complexes proposed to be useful for information storage and quantum information processing applications. In the quest for multilevel systems that can act as Qudits, two dysprosium-based isotopologues were synthesized and characterized. The isotopologues are [164Dy2(tmhd)6(tape)] (1(I=0)) and [163Dy2(tmhd)6(tape)] (2(I=5/2)), where tmhd = 2,2,6,6-tetramethylheptandionate and tape = 1,6,7,12-tetraazaperylene. Both complexes showed slow relaxation at a zero applied magnetic field with dominant Orbach and Raman relaxation mechanisms. μSQUID studies at milli-Kelvin temperatures reveal quasi-single ion loops, in contrast with the expected S-shape (near zero field) butterfly loops, characteristic of antiferromagnetically coupled dimeric complexes. Through analysis of the low-temperature data, we find that the interaction operating between Dy(III) is small, leading to a small exchange biasing from the zero-field transition. The resulting indirectly coupled nuclear states are degenerate or possess a small energy difference between them. We, therefore, conclude that for the creation of Qudits with enlarged Hilbert spaces, shorter Dy(III)···Dy(III) distances are deemed essential." @default.
• W4386346563 created "2023-09-02" @default.
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• W4386346563 date "2023-09-01" @default.
• W4386346563 modified "2023-10-01" @default.
• W4386346563 title "Hilbert Space in Isotopologue Dy(III) SMM Dimers: Dipole Interaction Limit in [^163/164Dy₂(tmhd)₆(tape)]⁰ Complexes" @default.
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• W4386346563 doi "https://doi.org/10.1021/acs.inorgchem.3c02246" @default.
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