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- W4386374829 abstract "In this study, a FeOCl adsorbent was demonstrated to rapidly remove perfluorocarboxylic acids (PFCAs). The unique coordination environment led to preferential dissociation of the Cl− in the FeOCl lattice by hydration, forming a high-intensity interfacial micro-electric field. The interfacial micro-electric field could apply an electric driving force to increase the external diffusion flux of PFCAs, thus achieving rapid adsorption (adsorption equilibrium time ∼10 min). In addition, the interfacial micro-electric field excited synergistic adsorption of multiple interactions (complexation, electrostatic interaction, and halogen-bonding interaction), being able to reach 277.01 mg/g for perfluorooctanoic acid (PFOA). Additionally, we developed a continuous flow column using FeOCl to demonstrate its potential for decontaminating drinking water with PFCAs at environmentally relevant concentrations. The FeOCl adsorbent exhibited excellent 125,000 BV to 70 ng/L breakthrough in dynamic adsorption experiments at high flow rates, which outperformed conventional activated carbon F400D and ion exchange resin IRA67 adsorbents. Spent FeOCl absorbent could be easily regenerated in mild regeneration conditions and maintained a high PFOA removal in subsequent usage cycles. FeOCl demonstrated great potential in the purification of PFCA-contaminated water for household or municipal applications." @default.
- W4386374829 created "2023-09-02" @default.
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- W4386374829 date "2023-12-01" @default.
- W4386374829 modified "2023-10-14" @default.
- W4386374829 title "Bio-inspired interfacial micro-electric field of FeOCl nanosheets for rapid adsorption of perfluorocarboxylic acids (PFCAs)" @default.
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- W4386374829 doi "https://doi.org/10.1016/j.seppur.2023.124980" @default.
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