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• W4386400635 abstract "Silicon (Si) has become the most promising next-generation anode to replace commercial graphite for Li-ion batteries (LIBs) profiting from its large reversible capacity of 4,200 mA h g-1. However, its sluggish reaction kinetics and large volume effect need to be resolved. Herein, we prepare a ternary GaSiP solid solution with a disordered lattice by a facile mechanochemistry method. As anodes of LIBs, the GaSiP provides a reversible capacity of 1,527 mA h g-1 at 100 mA g-1 with an initial Coulombic efficiency (ICE) of 90.8% based on the reversible Li-storage mechanism integrated intercalation and subsequent conversion processes as confirmed by crystallography characterization and electrochemical measurements. Importantly, the GaSiP carbon composite presents a long cycling stability of maintaining 1,362 mA h g-1 after 50 cycles at 0.1 A g-1, and 75% capacity retention rate after 1,200 cycles at 2 A g-1, and a high-rate performance of remaining 440 mA h g-1 at 20 A g-1. Broadly, this work opens the door to develop ternary phosphides with disordered lattice and liquid metallic phase using for electrochemical energy conversion and storage." @default.
• W4386400635 created "2023-09-04" @default.
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• W4386400635 date "2023-10-01" @default.
• W4386400635 modified "2023-10-18" @default.
• W4386400635 title "Disordered GaSiP Solid Solution Anodes with Liquid Metal Phase for High-Performance Li-Ion Batteries" @default.
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• W4386400635 doi "https://doi.org/10.1016/j.elecom.2023.107566" @default.
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