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- W4386415771 abstract "Every year vast quantities of silver are lost in various waste streams; this, combined with its limited, diminishing supply and rising demand, makes silver recovery of increasing importance. Thus, herein, we report a controllable, green process to produce a host of highly porous metal-organic framework (MOF)/oligomer composites using supercritical carbon dioxide (ScCO2 ) as a medium. One resulting composite, referred to as MIL-127/Poly-o-phenylenediamine (PoPD), has an excellent Ag+ adsorption capacity, removal efficiency (>99 %) and provides rapid Ag+ extraction in as little as 5 min from complex liquid matrices. Notably, the composite can also reduce sliver concentrations below the levels (<0.1 ppm) established by the United States Environmental Protection Agency. Using theoretical simulations, we find that there are spatially ordered polymeric units inside the MOF that promote the complexation of Ag+ over other common competing ions. Moreover, the oligomer is able to reduce silver to its metallic state, also providing antibacterial properties." @default.
- W4386415771 created "2023-09-05" @default.
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- W4386415771 date "2023-09-18" @default.
- W4386415771 modified "2023-10-15" @default.
- W4386415771 title "Rapid, Selective Extraction of Silver from Complex Water Matrices with a Metal‐Organic Framework/Oligomer Composite Constructed via Supercritical CO2" @default.
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- W4386415771 doi "https://doi.org/10.1002/anie.202309737" @default.
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