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- W4386444285 abstract "The topotactic intercalation of transition-metal dichalcogenides with atomic or molecular ions acts as an efficient knob to tune the electronic ground state of the host compound. A representative material in this sense is $1Ttext{ensuremath{-}}{mathrm{TiSe}}_{2}$, where the electric-field-controlled intercalations of lithium or hydrogen trigger superconductivity coexisting with the charge-density-wave phase. Here, we use the nuclear magnetic moments of the intercalants in hydrogen-intercalated $1Ttext{ensuremath{-}}{mathrm{TiSe}}_{2}$ as local probes for nuclear magnetic resonance experiments. We argue that fluctuating mesoscopic-sized domains nucleate already at temperatures higher than the bulk critical temperature to the charge-density-wave phase and display cluster-glass-like dynamics in the MHz range tracked by $^{1}mathrm{H}$ nuclear moments. Additionally, we observe a well-defined independent dynamical process at lower temperatures that we associate with the intrinsic properties of the charge-density-wave state. In particular, we ascribe the low-temperature phenomenology to the collective phasonlike motion of the charge-density wave being hindered by structural defects and chemical impurities and resulting in a localized oscillating motion." @default.
- W4386444285 created "2023-09-06" @default.
- W4386444285 creator A5005493217 @default.
- W4386444285 creator A5026549682 @default.
- W4386444285 creator A5051087387 @default.
- W4386444285 creator A5073389861 @default.
- W4386444285 creator A5074768738 @default.
- W4386444285 date "2023-09-05" @default.
- W4386444285 modified "2023-09-27" @default.
- W4386444285 title "Cluster charge-density-wave glass in hydrogen-intercalated <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi>TiSe</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>" @default.
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