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- W4386460147 abstract "Abstract Low‐cost and on‐site H 2 O 2 production is desirable for industrial and civilian usage. (Photo)electrochemical H 2 O 2 production is proposed to be a safer, greener, and cheaper strategy for on‐site H 2 O 2 production as compared to the conventional anthraquinone process and the direct thermal synthesis. However, the efficiency, selectivity, and durability of the (photo)electrochemical H 2 O 2 production devices are still not satisfactory. Therefore, there is an urgent need to revisit the (photo)electrocatalyst and device designs for (photo)electrochemical on‐site H 2 O 2 production, thus to rationalize the research thoughts and provide valuable guidance. This review comprehensively summarizes and discusses the mechanism of two‐electron oxygen reduction reaction (2e − ORR) and two‐electron water oxidation reaction (2e − WOR) for H 2 O 2 production, and the current research status on the (photo)electrocatalysts and (photo)electrochemical devices. In particular, the pros and cons of the four types of (photo)electrochemical device designs, which are Type I (2e − ORR + oxygen evolution reaction), Type II (2e − ORR + hydrogen oxidation reaction), Type III (2e − WOR + hydrogen evolution reaction) and Type IV (2e − WOR + 2e − ORR), are discussed in detail. Finally, a practical perspective on the future research directions for the on‐site (photo)electrochemical H 2 O 2 production based on the technical challenges of this technique is provided." @default.
- W4386460147 created "2023-09-06" @default.
- W4386460147 creator A5006901857 @default.
- W4386460147 creator A5015195367 @default.
- W4386460147 creator A5021163747 @default.
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- W4386460147 creator A5051085470 @default.
- W4386460147 creator A5058533540 @default.
- W4386460147 creator A5073108451 @default.
- W4386460147 creator A5082016278 @default.
- W4386460147 creator A5082971300 @default.
- W4386460147 date "2023-09-04" @default.
- W4386460147 modified "2023-09-27" @default.
- W4386460147 title "Recent Progress on the Catalysts and Device Designs for (Photo)Electrochemical On‐Site H<sub>2</sub>O<sub>2</sub> Production" @default.
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