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- W4386561907 abstract "Environmental pollution is one of the main challenges currently faced by mankind; especially industrial waste-waters treatment and remediation using energy-efficient methodologies. This research focused on the electrochemical degradation of the hazardous nitrobenzene (NB) in aqueous solutions, using novel high-entropy oxide (HEO) electrodes to elucidate the influence of the electrochemical reduction step on the degradation process. The effect of solution pH, dissolved oxygen concentration, anodic applied potential, and cell configurations on NB hydrogenation reaction were evaluated. A synergistic effect between the hydrogenation of nitrobenzene and the degradation was found to drastically enhance the conversion rates. The presence of dissolved oxygen promoted the oxidation reactions, reaching more than 90% nitrobenzene removal at 1.7 V and pH 14. The degradation of the organic by-products was attributed to the formation of the superoxide radical (O2*-) as the main oxidant species. A degradation mechanism was proposed based on the detected intermediates and the decoupling of electrochemical surface reactions observed by EIS at different solution pH." @default.
- W4386561907 created "2023-09-09" @default.
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- W4386561907 date "2023-11-01" @default.
- W4386561907 modified "2023-10-16" @default.
- W4386561907 title "Evaluation of the hydrogenation reaction on the electrocatalytic nitrobenzene degradation over (FeCoNiCuZn)xOy high entropy oxides (HEOs)" @default.
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- W4386561907 doi "https://doi.org/10.1016/j.chemosphere.2023.140130" @default.
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- W4386561907 hasPublicationYear "2023" @default.
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