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- W4386573383 abstract "The effect of halide ion on the catalytic activity for the aqueous-phase partial oxidation of methane with H2O2 generated in situ over Pd/C was examined. Various halide ions, including F-, Cl-, Br-, and I- were compared. Among them, Br- and I- are effective for the synthesis of H2O2 from H2 and O2, resulting in the synthesis of methane oxygenates from methane over Fe/ZSM-5. They show different product yields as a function of their concentrations. The highest total product yields were obtained with [KBr] = 5 mM and [KI] = 0.05 mM, respectively. Compared with Br-, the highest product yield was obtained with a much lower concentration of I-, guaranteeing that no detectable leaching of metal from Fe/ZSM-5 and Pd/C was found. The total productivity was 4.64 mmol/gcat./h over Fe/ZSM-5 at 50 ℃ with H2O2 generated in situ over Pd/C from H2 and O2 in the presence of 0.05 mM of KI." @default.
- W4386573383 created "2023-09-10" @default.
- W4386573383 creator A5008033127 @default.
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- W4386573383 date "2024-01-01" @default.
- W4386573383 modified "2023-09-27" @default.
- W4386573383 title "Partial oxidation of methane over Fe/ZSM-5 with hydrogen peroxide generated in situ over Pd/C in the presence of halide ions" @default.
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- W4386573383 doi "https://doi.org/10.1016/j.cattod.2023.114367" @default.
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