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- W4386573584 abstract "Catalytic fixed-bed is an efficient and facile system for scalable organic synthesis due to its continuous and fast flow operation process. As a key unit in the fixed-bed system, catalytically active packing materials are required to possess some properties, such as high activity, excellent stability, and porous packing structure. Herein, we prepare a fibrous fixed-bed catalyst by anchoring Pd nanoparticles on N-doped graphene fiber (NHG) (Pd/NGF). Due to the porous and loose packing structure, the resultant Pd/NGF catalyst can be easily filled into the continuous-flow reactor to construct a fixed-bed system with low flow resistance. The corresponding catalytic fixed-bed system exhibits a favourable flow rate (8 mL/min) and excellent durability toward reduction reactions of N-containing unsaturated compounds to produce aromatic amines. This work provides a new design concept of fibrous fixed-bed catalysts with dual-active components (i.e., graphene-derived active materials and metal nanoparticles) and catalytic organic synthesis in a continuous-flow process." @default.
- W4386573584 created "2023-09-10" @default.
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- W4386573584 date "2023-09-01" @default.
- W4386573584 modified "2023-09-26" @default.
- W4386573584 title "N-doped graphene fiber anchored Pd nanoparticles as a fixed-bed catalyst for continuous-flow reduction of N-containing unsaturated compounds" @default.
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- W4386573584 doi "https://doi.org/10.1016/j.gresc.2023.08.003" @default.
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