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• W4386575333 abstract "The all-solid-state lithium batteries (ASSLBs) with high energy density are considered to be one of the most promising candidates for next-generation lithium battery systems. Nevertheless, the low ionic and electronic conduction inside the cathode and the poor interfacial contact of the cathode/electrolyte seriously impede the large-scale application of ASSLBs. In this work, a novel multiple ion-electron conductive network is constructed on the FeS2 cathode to realize a high-energy all-solid-state battery. The internal disordered carbon matrix acts as electronic network to accelerate the electronic transmission. Meanwhile, reduced graphene oxide (rGO) tightly wrapping FeS2/C microspheres' surface serves as external electronic pathway. Moreover, the in-situ formed Li7P3S11 electrolyte infiltrates into the nanoparticles to improve lithium-ion transport kinetics. Therefore, the dual-carbon framework and Li7P3S11 coating layer strategies significantly enhance ion-electron transport kinetics and improve interfacial contact during cycling. As expected, the FeS2@C/rGO@Li7P3S11 cathode exhibits excellent rate capability and cycling stability, showing a reversible discharge capacity of 350.3 mAh/g at 0.5C after 200 cycles. More importantly, ex-situ XPS and dQ/dV results reveal that the synergistic effect of dual-carbon frameworks and Li7P3S11 coating layer not only provides fast electron-ion transfer channels, but also wraps the reaction products with poor electrochemical activity such as Fe0, FeSy, and S to accelerate the reaction kinetics and strengthens the reaction reversibility. This work provides valuable insights for improving the electrochemical performance and understanding the reaction mechanism of the conversion-type metal sulfide cathodes in ASSLBs." @default.
• W4386575333 created "2023-09-10" @default.
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• W4386575333 date "2024-01-01" @default.
• W4386575333 modified "2023-10-16" @default.
• W4386575333 title "Construction of ion-electron conduction network on FeS2 as high-performance cathodes enables all-solid-state lithium batteries" @default.
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• W4386575333 doi "https://doi.org/10.1016/j.jcis.2023.09.048" @default.
• W4386575333 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37708735" @default.
• W4386575333 hasPublicationYear "2024" @default.
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