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• W4386600389 endingPage "115152" @default.
• W4386600389 startingPage "115152" @default.
• W4386600389 abstract "The present work exemplifies MOF as a unique functional scaffold for ultrasensitive monitoring of L-Arginine (Arg) over L-Lysine (Lys) and other amino acids from purely aqueous medium. In this context, a thermostable ZnII-functionalized MOF (viz. ZnII-CA-LMOF) has been synthesized utilizing α-hydroxy acid containing aliphatic ligand like citric acid (CA). The MOF provides an excellent platform for optical speciation of Arg over other competitive biohazards via “turn-on” fluorescence response with a limit of detection 3.3 ppb (R = 0.99) with response time of ∼90 s. Interestingly, the Zn-MOF has been exploited for detecting Arg from complex bio-fluids which are of immense clinical importance. Additionally, DFT studies shed light on the role of SBUs in non-covalent interaction between CA and targeted bio-hazards in a confined space which results in desired molecular sieving amongst different bio-analytes. Moreover, the host–guest interactions through “turn-off-on-off” have been utilized for fabricating molecular electronics. In brief, the demand of formulizing a single platform to rationalize the structure-performance synergies to fabricate smarter material has been properly emphasized in the current work." @default.
• W4386600389 created "2023-09-12" @default.
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• W4386600389 date "2024-01-01" @default.
• W4386600389 modified "2023-10-05" @default.
• W4386600389 title "Molecular sieving of L-arginine over l-Lysine by α-Hydroxy acid functionalized ZnII-luminescent framework from aqueous medium and other biofluids: Experimental and DFT corroboration with logic gate construction" @default.
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• W4386600389 doi "https://doi.org/10.1016/j.jphotochem.2023.115152" @default.
• W4386600389 hasPublicationYear "2024" @default.
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