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- W4386609459 abstract "The shuttle effect and sluggish redox kinetics of sulfur cathode are the main barriers to commercializing lithium-sulfur (Li-S) batteries. Fabricating functional interlayers is considered as one of the efficient approaches to suppress the shuttle effect while accelerating the conversion kinetics of polysulfides. Herein, the nanofiber-type interlayer composed of cobalt wrapped with few-layer phosphorus-doped graphite (CoPG) is elaborately designed, which is expected to chemically adsorb the polysulfides while accelerating the redox conversion of polysulfides anchored on phosphorus-doped graphite. Electrochemical measurements sufficiently verify that the usage of the designed CoPG interlayer significantly prolongs the longevity of Li-S batteries, reaching 694 mAh g-1 with a capacity decay rate of 0.11% at the current density of 2.0 C. Remarkably, Li-S battery sustains for 125 cycles and maintains ultrahigh capacity retention of 92% at the current density of 0.2 C even with a sulfur loading of 5.8 mg cm-2. The theoretical computation further confirms the intensive interactions between CoPG and polysulfides, consistent with the experimental outcomes. Encapsulating the electrocatalyst with a few-layer polarized graphite enables the interlayer with adsorption and catalysis functions, which provides a promising strategy for advanced Li-S batteries." @default.
- W4386609459 created "2023-09-12" @default.
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- W4386609459 date "2023-10-01" @default.
- W4386609459 modified "2023-10-17" @default.
- W4386609459 title "Phosphorus-doped Few-layer Graphite Wrapped Metallic Cobalt as Interlayer for Advanced Lithium-Sulfur Batteries" @default.
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- W4386609459 doi "https://doi.org/10.1016/j.mtener.2023.101415" @default.
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