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• W4386630006 abstract "The exploration of advanced materials through rational structure/phase design is the key to develop high-performance lithium-ion capacitors (LICs). However, high complexity of material preparation and difficulty in quantity production largely hinder the further development. Herein, Cu5FeS4-x/C (CFS@C) heterojunction with rich sulfur vacancies has successfully achieved from natural bornite, presenting low cost-effective and bulk-production prospect. Density functional theory calculations (DFT) indicate that rich vacancies in bulk phase can decrease band gap of bornite and thus improve its intrinsic electron conductivity, as well as the heterojunction spontaneously evokes a built-in electric field between its interfacial region, largely reducing the migration barrier from 1.27 eV to 0.75 eV. Benefited from these merits, the CFS@C electrodes deliver outperformed lithium storage performance, e.g., high reversible capacity (822.4 mAh/g at 0.1 A/g), excellent cycling stability (up to 820 cycles at 2 A/g and 540 cycles at 5 A/g with respective capacity retention of over or nearly 100%). With CFS@C as anode and porous carbon nanosheets (PCS) as cathode, the assembled CFS@C//PCS LIC full cells exhibit high energy/power density characteristics of 139.2 Wh/kg at 2500 W/kg. This work is expected to offer significant insights into structure modifications/devising toward natural minerals for advanced energy-storage systems." @default.
• W4386630006 created "2023-09-13" @default.
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• W4386630006 date "2023-09-01" @default.
• W4386630006 modified "2023-10-18" @default.
• W4386630006 title "Interfacial/bulk synergetic effects accelerating charge transferring for advanced lithium-ion capacitors" @default.
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• W4386630006 doi "https://doi.org/10.1016/j.cclet.2023.109081" @default.
• W4386630006 hasPublicationYear "2023" @default.
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