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• W4386754695 abstract "We have studied the stability of the smallest long-lived all carbon molecular dianion (C_{7}^{2-}) in new time domains and with a single ion at a time using a cryogenic electrostatic ion-beam storage ring. We observe spontaneous electron emission from internally excited dianions on millisecond timescales and monitor the survival of single colder C_{7}^{2-} molecules on much longer timescales. We find that their intrinsic lifetime exceeds several minutes-6 orders of magnitude longer than established from earlier experiments on C_{7}^{2-}. This is consistent with our calculations of vertical electron detachment energies predicting one inherently stable isomer and one isomer which is stable or effectively stable behind a large Coulomb barrier for C_{7}^{2-}→C_{7}^{-}+e^{-} separation." @default.
• W4386754695 created "2023-09-15" @default.
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• W4386754695 date "2023-09-13" @default.
• W4386754695 modified "2023-10-14" @default.
• W4386754695 title "Stability and Cooling of the <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msubsup><mml:mrow><mml:mi mathvariant=normal>C</mml:mi></mml:mrow><mml:mrow><mml:mn>7</mml:mn></mml:mrow><mml:mrow><mml:mn>2</mml:mn><mml:mo>−</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math> Dianion" @default.
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• W4386754695 doi "https://doi.org/10.1103/physrevlett.131.113003" @default.
• W4386754695 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37774298" @default.
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