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- W4386764980 abstract "Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light-matter interaction was, so far, not studied systematically at free-electron lasers-its dependence on the photon energy. Here, we use resonant ion spectroscopy to map out the transient electronic structures occurring during the complex charge-up pathways of xenon. Massively hollow atoms featuring up to six simultaneous core holes determine the spectra at specific photon energies and charge states. We also illustrate how different X-ray pulse parameters, which are usually intertwined, can be partially disentangled. The extraction of resonance spectra is facilitated by the possibility of working with a constant number of photons per X-ray pulse at all photon energies and the fact that the ion yields become independent of the peak fluence beyond a saturation point. Our study lays the groundwork for spectroscopic investigations of transient atomic species in exotic, multiple-core-hole states that have not been explored previously." @default.
- W4386764980 created "2023-09-16" @default.
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- W4386764980 date "2023-09-15" @default.
- W4386764980 modified "2023-10-12" @default.
- W4386764980 title "Multiple-core-hole resonance spectroscopy with ultraintense X-ray pulses" @default.
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- W4386764980 doi "https://doi.org/10.1038/s41467-023-41505-1" @default.
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