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• W4386815904 abstract "One-step phenol hydrogenation over Pd@N-doped carbon (CN) is a sustainable approach to produce cyclohexanone, a key intermediate in the production of nylon. In this work, cobalt sources and 2-methylimidazole (2-MeIm) were mixed and directly carbonized to synthesize CN materials. After acid etching and Pd loading, the Pd2+@CN catalysts were achieved, and the porous structures and surface properties can be modulated by tuning the kind of cobalt sources and the molar ratio of 2-MeIm and cobalt. The Pd2+@CN(D) (prepared by the direct carbonization strategy) demonstrates comparable performance in the phenol hydrogenation to the ZIF-67-derived Pd2+@CN(67), and more importantly, the obtained weight of Pd2+@CN(D) is 2.1 times higher than that of Pd2+@CN(67). The optimum Pd2+@CN-4 (synthesized with a molar ratio of 4 between 2-MeIm and cobalt acetate tetrahydrate) achieves superior and durable catalytic performance (a turnover frequency (TOF) of 125.9 h−1) for the well-developed hierarchically porous structures, rich defects and abundant alkaline." @default.
• W4386815904 created "2023-09-18" @default.
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• W4386815904 date "2023-09-01" @default.
• W4386815904 modified "2023-10-15" @default.
• W4386815904 title "Facile and efficient synthesis of Pd2+@CN catalysts for enhanced phenol hydrogenation to cyclohexanone" @default.
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• W4386815904 doi "https://doi.org/10.1016/j.apcata.2023.119428" @default.
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