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- W4386853078 abstract "Gas diffusion electrodes are essential components of common fuel and electrolysis cells that use gas phase reactants and products, but are typically made from graphitic carbon or metallic materials, which do not allow light transmittance, and thus limit the development of photoelectrode membrane assemblies for gas-phase solar fuel production. In this presentation, the application of solar H 2 production from humid air is motivated and the simple and scalable preparation of transparent gas-diffusion layers using F-doped SnO 2 (FTO) coated SiO 2 interconnected fiber felt substrates is introduced. The resulting substrates have a porosity of 90 %, a roughness factor of 15.8 and a Young’s Modulus of 0.2 GPa. A sheet resistivity of 20 ± 3 Ω sq−1 and a loss of incident light of 41% at an illumination wavelength of 550 nm is found with FTO coating. The application of various semiconductors on the substrates was established including Fe2O3 (chemical bath deposition), CuSCN and Cu2O (electrodeposition), and semiconducting polymers (dip coating) and the liquid-phase photoelectrochemical performance commensurate with flat FTO substrates was confirmed. Finally, gas phase H 2 production was demonstrated with a polymer semiconductor photocathode membrane assembly at 1-Sun photocurrent density on the order of 1 mA cm –2 and Faradaic efficiency of 40%." @default.
- W4386853078 created "2023-09-20" @default.
- W4386853078 creator A5036944455 @default.
- W4386853078 date "2023-08-28" @default.
- W4386853078 modified "2023-10-02" @default.
- W4386853078 title "(Invited) Photoelectrode Membrane Assemblies with Transparent Conductive Gas Diffusion Layers for Solar Fuel Production" @default.
- W4386853078 doi "https://doi.org/10.1149/ma2023-01372142mtgabs" @default.
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