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• W4386855849 abstract "The synthesis and utilization of defect-rich biomass carbon catalysts with varying Co concentrations and incorporated Ce in CH4-CO2 reforming were investigated. The catalytic performance of these catalysts was found to increase with higher Co content, reaching its optimum at a Co concentration of 20 %. The presence of Ce as a promoter improved the utilization of Co precursors and enhanced the dispersion of Co sites at defective structures on the catalyst surface. The confined space within the defective structures restricted the growth of Co particles, resulting in smaller and more uniformly dispersed Co particles on the catalyst surface. Additionally, the introduction of Ce species influenced the oxygen environment on the catalyst surface. XPS analysis confirmed that the addition of Ce led to an increase in the chemisorbed oxygen content, enhancing the catalyst's ability to activate CO2. The increased percentage of chemisorbed oxygen, coupled with improved CO2 activation capacity, contributed to the Co-Ce bimetallic catalyst's ability to resist carbon deposition. The Co-Ce bimetallic catalyst demonstrated exceptional stability and performance in CH4-CO2 reforming due to its enhanced metal dispersion, reduced metal particle size, and improved CO2 activation capacity. The incorporation of Ce as a promoter played a crucial role in achieving these desirable catalytic properties." @default.
• W4386855849 created "2023-09-20" @default.
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• W4386855849 date "2023-11-01" @default.
• W4386855849 modified "2023-10-13" @default.
• W4386855849 title "Co-based defect-rich nanoarchitectonics with biomass carbon materials catalysts for CH4–CO2 reforming" @default.
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• W4386855849 doi "https://doi.org/10.1016/j.mcat.2023.113566" @default.
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