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- W4386870210 abstract "The reduction of [CoLBr2], a CoII complex supported by a diisopropylphosphinoquinoline (L) ligand, induced a ligand coupling giving access to a (PNNP) supported CoII complex which was isolated in 70% yield. This complex was formed using a minimum of 2 equivalents of a reductant (either Mn or KC8). The fate of [CoLBr2] in the presence of 1 equivalent of a reductant was more difficult to study; nevertheless, a CoI complex was characterised in the solid state. In order to determine whether this ligand coupling could occur with other 3d metals, L supported FeII and NiII complexes were synthesised. While no compound could be identified upon reduction of [FeLBr2], both [NiLBr2] and [NiL2Br](Br) led to the reduction at the metal center allowing the isolation of an original Ni0 trimer in a satisfactory yield. This study shows the different behaviours of these 3d metal complexes in the presence of a reductant." @default.
- W4386870210 created "2023-09-20" @default.
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- W4386870210 date "2023-01-01" @default.
- W4386870210 modified "2023-10-06" @default.
- W4386870210 title "Phosphinoquinoline supported CoII, NiII, and FeII complexes: divergent behaviour upon reduction" @default.
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- W4386870210 doi "https://doi.org/10.1039/d3dt02441e" @default.
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