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- W4386872214 abstract "Hydrogenation of palm oil over commercial NiMo/γ-Al2O3 catalysts and the effect of operating conditions were investigated in an autoclave with a continuous H2 flow mode. Methanation as the side reactions were taken into account in the reaction path selectivity for the first time. Three competing reaction pathways of hydrodecarboxylation, hydrocarbonation, and direct hydrodeoxygenation were clearly distinguished by quantifying the oxygen in the aqueous, organic, and gas phases. The results corroborated that the temperature and hydrogen supply were crucial to oxygen removal and the selectivity of the HDO pathways. Methane is the predominant gas product rather than propane during triglyceride deoxygenation, in which 87–100% of the methane production comes from the glycerol skeleton of the triglyceride and the rest comes from the CO methanation. Lower temperature favored the direct HDO route, while the selectivity of the HDCO and HDCO2 reactions preferred a higher temperature. HDO dominated the hydrodeoxygenation process under all H2 supply conditions, followed by the HDCO2 pathway and the HDCO reaction. This study brings the understanding of the vegetable oil triglyceride hydrodeoxygenation process to the molecular level and can potentially guide the optimization of process conditions." @default.
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- W4386872214 date "2023-12-01" @default.
- W4386872214 modified "2023-09-27" @default.
- W4386872214 title "Analysis of palm oil hydrodeoxygenation pathway selectivity based on oxygen quantification" @default.
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- W4386872214 doi "https://doi.org/10.1016/j.fuproc.2023.107950" @default.
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