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• W4386959619 endingPage "125169" @default.
• W4386959619 startingPage "125169" @default.
• W4386959619 abstract "Materials with high adsorption properties and high selectivity are ideal adsorbents for the application of adsorption. Herein, by using tetrabrombisphenol A (TBr-BPA) as the template, a novel COF-based composite (SiO2@F-COF@MIP) with directional selectivity and three-dimensional spatial selectivity was developed for the first time. Superior selective adsorption effects of TBr-BPA and family-similar compound (tetrachlorbisphenol, TCl-BPA) can be achieved by using composite as the adsorbent. Firstly, to verify the performance of the composite, the selective adsorption effects of F-COF, SiO2-NH2, SiO2-NH2@F-COF and SiO2@F-COF@MIP on TBr-BPA, TCl-BPA and competing compounds were investigated and compared. Results showed that SiO2@F-COF@MIP had extremely high selective adsorption capacities for TBr-BPA and TCl-BPA with the maximal adsorption capacities of 653.2 and 158.8 mg·g−1, respectively. Secondly, by using computer simulation and experiments analysis, the mechanisms of SiO2@F-COF@MIP for the highly selective adsorption were explored. Results revealed the selective adsorption of TBr-BPA on SiO2@F-COF@MIP was mainly based on halogen bond interaction, three-dimensional space selectivity effect coupled with hydrogen bond and electrostatic interactions. The selective adsorption of TCl-BPA was mainly based on three-dimensional space selectivity, hydrogen bond and electrostatic interactions. Finally, SiO2@F-COF@MIP was used as the adsorbent for the enrichment of TBr-BPA and TCl-BPA in actual water and fish samples, and satisfactory recoveries were obtained, proving that SiO2@F-COF@MIP has great application prospect in high selective enrichment." @default.
• W4386959619 created "2023-09-23" @default.
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• W4386959619 date "2024-01-01" @default.
• W4386959619 modified "2023-09-30" @default.
• W4386959619 title "Fusion of materials with directional-selection and family-selection properties to prepare covalent organic framework composite with superior selective adsorption performance" @default.
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• W4386959619 doi "https://doi.org/10.1016/j.seppur.2023.125169" @default.
• W4386959619 hasPublicationYear "2024" @default.
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