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• W4387003105 abstract "Infrared reflection absorption spectroscopy (IRRAS) is commonly used to study the structure and chemistry of molecules residing at surfaces, including water surfaces, which has far-reaching applications including atmospheric chemistry and food science. However, there is some debate regarding the surface-specificity of IRRAS when examining soluble surfactants on aqueous solutions, and there is some evidence that the surface-specificity may differ between IRRAS of ionic surfactants and soluble organic acids. This paper presents infrared reflection absorption (IRRA) spectra of soluble organic acids underneath monolayers of insoluble surfactants, where the contributions from the insoluble surfactants are subtracted from the spectra to capture subsurface effects. These subsurface spectra demonstrate that IRRA spectra of soluble organic acids are surface specific, and this observation is supported by a simplified model for reflections from subsurface layers. Finally, the observations presented here are compared to literature observations regarding the surface-specificity of IRRAS when studying ionic surfactants. Overall, this work demonstrates the utility of IRRAS for studying the structures and chemistry of soluble organic acids at aqueous surfaces." @default.
• W4387003105 created "2023-09-26" @default.
• W4387003105 creator A5088239798 @default.
• W4387003105 date "2023-09-25" @default.
• W4387003105 modified "2023-10-01" @default.
• W4387003105 title "Infrared Reflection Absorption Spectroscopy (IRRAS) of Water-Soluble Surfactants: Is it Surface-Specific?" @default.
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• W4387003105 doi "https://doi.org/10.1177/00037028231200903" @default.
• W4387003105 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37743797" @default.
• W4387003105 hasPublicationYear "2023" @default.
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