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• W4387007573 abstract "The integration of electronic effects into complexes for the construction of novel materials has not yet attracted significant attention in the field of energy storage. In the current study, eight one-dimensional (1D) nickel-based salicylic acid (SA) complexes, Ni-XSAs (X = pH, pMe, pMeO, mMe, pBr, pCl, pF, and pCF3 ), are prepared by ligand engineering. The coordination environments in the Ni-XSAs are explored using X-ray absorption fine structure (XAFS) spectroscopy. The charge transfer of the complexes is modulated according to the difference in the electron-donating ability of the substituents, in combination with frontier orbital theory. Furthermore, density functional theory (DFT) is used to investigate the effect of the substituent position on the electronic properties of the complexes. Ni-mMeSA exhibits better electrical conductivity than Ni-pMeSA. The electrochemical performance of Ni-mMeSA as an aqueous battery cathode is remarkably improved with a maximum energy density of 0.30 mWh cm-2 (125.00 Wh kg-1 ) and a peak power density of 33.72 mW cm-2 (14.03 kW kg-1 ). This study provides ideas for the application of new coordination chemistry in the field of energy materials science. This article is protected by copyright. All rights reserved." @default.
• W4387007573 created "2023-09-26" @default.
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• W4387007573 date "2023-09-25" @default.
• W4387007573 modified "2023-09-27" @default.
• W4387007573 title "Regulating Intramolecular Electron Transfer of Nickel‐Based Coordinations through Ligand Engineering for Aqueous Batteries" @default.
• W4387007573 doi "https://doi.org/10.1002/adma.202307003" @default.
• W4387007573 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37748200" @default.
• W4387007573 hasPublicationYear "2023" @default.
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