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- W4387012324 abstract "Electron-vibration coupling is of critical importance for the development of molecular electronics, spintronics, and quantum technologies, as it affects transport properties and spin dynamics. The control over charge-state transitions and subsequent molecular vibrations using scanning tunneling microscopy typically requires the use of a decoupling layer. Here we show the vibronic excitations of tetrabromotetraazapyrene (TBTAP) molecules directly adsorbed on Ag(111) into an orientational glassy phase. The electron-deficient TBTAP is singly-occupied by an electron donated from the substrate, resulting in a spin 1/2 state, which is confirmed by a Kondo resonance. The TBTAP•- discharge is controlled by tip-gating and leads to a series of peaks in scanning tunneling spectroscopy. These occurrences are explained by combining a double-barrier tunneling junction with a Franck-Condon model including molecular vibrational modes. This work demonstrates that suitable precursor design enables gate-dependent vibrational excitations of molecules on a metal, thereby providing a method to investigate electron-vibration coupling in molecular assemblies without a decoupling layer." @default.
- W4387012324 created "2023-09-26" @default.
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- W4387012324 date "2023-09-25" @default.
- W4387012324 modified "2023-09-27" @default.
- W4387012324 title "Strong signature of electron-vibration coupling in molecules on Ag(111) triggered by tip-gated discharging" @default.
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- W4387012324 doi "https://doi.org/10.1038/s41467-023-41601-2" @default.
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