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- W4387036073 abstract "Cobalt-based catalysts have displayed intrinsic activity for selective hydrogenolysis of furfural alcohol (FFA) to 1,5-pentanediol (1,5-PDO), but how to efficiently enhance 1,5-PDO selectivity remain a challenge. We prepared a series of CoPtLa-Hx catalysts by different reduction temperatures, and found the interfacial synergy within the bimetallic oxide CoOx-PtOx of the CoPtLa-H5 catalyst not only boosted the dispersion of Co species and Pt species, also increased electronic interactions within the bimetallic oxide which promoted the formation of the content of Co2+ that are critical to C-O bond rupture of FFA. The interfacial synergy significantly enhanced the 1,5-PDO yield (40.3 %) and favored high catalyst stability. We found that the formations of 1,5-PDO, 1,2-PDO and tetrahydrofurfuryl alcohol (THFA) are competing reactions, which is helpful to the design of highly selective catalysts towards the conversion FFA to 1,5-PDO." @default.
- W4387036073 created "2023-09-27" @default.
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- W4387036073 date "2024-01-01" @default.
- W4387036073 modified "2023-10-15" @default.
- W4387036073 title "Interfacial synergy within bimetallic oxide promotes selective hydrogenolysis of furfuryl alcohol to 1,5-pentanediol" @default.
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- W4387036073 doi "https://doi.org/10.1016/j.apsusc.2023.158571" @default.
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