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• W4387169265 abstract "Abstract Electrochemical reduction of CO 2 is widely researched in recent years. However, direct electro‐reduction of diluted CO 2 to C 2 products is seldomly studied. In this work, electrocatalytic reduction of CO 2 with different concentrations were conducted on Cu 2 (PO 4 )(OH) catalysts. The catalytic performance in diluted CO 2 is comparable with that in pure CO 2 by using Cu 2 (PO 4 )(OH) as catalyst. Besides, the selectivity of C 2 product is still as high as 64.6% in 50%CO 2 concentration. The normalized C 2 current density of Cu 2 (PO 4 )(OH) was over 6.8 times higher than that of commonly used Cu 2 O–Cu catalyst with similar size. In situ Raman spectroscopy proved that Cu + is the main active site at higher potentials. More importantly, a higher local pH is realized under diluted CO 2 test conditions which is favorable for promoting C–C coupling. Finally, in situ ATR‐FTIR spectroscopy was performed to further monitor and identify the adsorbed intermediates and help reveal the mechanism for the catalysts." @default.
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• W4387169265 date "2023-09-29" @default.
• W4387169265 modified "2023-10-17" @default.
• W4387169265 title "Direct reduction of diluted <scp>CO₂</scp> gas to <scp>C₂</scp> products by copper hydroxyphosphate microrods" @default.
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• W4387169265 doi "https://doi.org/10.1002/aic.18233" @default.
• W4387169265 hasPublicationYear "2023" @default.
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