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- W4387213879 abstract "The exploration of high-performance benzoxazine thermosets from easily processable monomers is still a challenge with the enhancement on the concept of sustainable development from worldwide. In this contribution, a new bio-based benzoxazine monomer (DA-FBz) with two functionality was successfully prepared from renewable trans-anethole and furfurylamine. DA-FBz showed a low melting temperature (Tm) of 60 °C and could be easily converted into polybenzoxazine (poly(DA-FBz)) through ring-opening thermal polymerization. The curing behavior was characterized by differential scanning calorimetry (DSC) and Fourier transform infrared (FT-IR) analysis. After thermal curing, the obtained poly(DA-FBz) exhibited high thermal stability with a 5 wt% loss temperature of 404 °C. In particular, this thermoset showed a high glass transition temperature of 334 °C due to the high crosslinking density constructed from the reactive furan structure during thermal polymerization. In addition, poly(DA-FBz) also exhibited high thermal mechanical strength with a storage modulus of 3 GPa at room temperature, which was still up to 1.2 GPa at 300 °C. This highly crosslinked framework also resulted into a low thermal expansion and low water absorption. All these results indicated this polybenzoxazine would be potential candidate used in high-performance engineering applications." @default.
- W4387213879 created "2023-10-01" @default.
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- W4387213879 date "2023-11-01" @default.
- W4387213879 modified "2023-10-09" @default.
- W4387213879 title "High-Tg bio-based polybenzoxazine derived from renewable anethole and furfurylamine" @default.
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- W4387213879 doi "https://doi.org/10.1016/j.eurpolymj.2023.112466" @default.
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