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• W4387241479 abstract "This article presents a comprehensive study on the synthesis and structural and thermal conductivity properties of cesium-inserted chromium tellurides of formula CsxCr5Te8. Single crystals of three different compositions (x = 0.73, 0.91, and 0.97) were successfully synthesized and suggested the existence of a solid solution in the range 0.73 < x < 1. Through a detailed single-crystal characterization, the complete structure of these compounds is determined, revealing a distinct B-type hollandite-like structural form derived from the hollandite structure, in contrast to the more commonly observed A-type pseudo-hollandite in AM5X8-type chalcogenides (A = cation, M = transition metal, and X = chalcogen). Periodic density functional theory calculations predict the Cs0.73Cr5Te8 composition as the most stable, with a metallic conductive behavior. The thermal conductivity of bulk CsxCr5Te8 samples is measured to be 1.4 W m-1 K-1 at 300 K and increases with temperature up to 2 W m-1 K-1 at 673 K." @default.
• W4387241479 created "2023-10-03" @default.
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• W4387241479 date "2023-10-02" @default.
• W4387241479 modified "2023-10-18" @default.
• W4387241479 title "Synthesis, Crystal and Electronic Structure, and Thermal Conductivity Investigation of the Hollandite-like Cs_<i>x</i>Cr₅Te₈ Phases (0.73 < <i>x</i> < 1)" @default.
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• W4387241479 doi "https://doi.org/10.1021/acs.inorgchem.3c02590" @default.
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• W4387241479 hasPublicationYear "2023" @default.
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